Dimethyl sulfide and its oxidation products in the atmosphere of the Atlantic and southern oceans

B. Davison, C. O'Dowd, C. N. Hewitt, M. H. Smith, R. M. Harrison, D. A. Peel, E. Wolf, R. Mulvaney, M. Schwikowski, U. Baltensperger

Research output: Contribution to a Journal (Peer & Non Peer)Conference articlepeer-review

47 Citations (Scopus)

Abstract

Dimethyl sulfide, methane sulfonate, non-sea-salt sulfate and sulfur dioxide concentrations in air were obtained during a cruise between the U.K. and the Antarctic during the period October 1992-January 1993. In equatorial regions (30°N to 30°S) the atmospheric DMS concentration ranged from 3 to 46 ng(S)m-3 with an average of 18 ng(S)m-3. In the polar waters and regions south of the Falkland Islands concentrations from 3 to 714 ng(S)m-3 were observed with a mean concentration of 73 ng(S)m-3 Methane sulfonate concentrations were also enhanced in the vicinity of the Antarctic Peninsula and in the Weddell Sea. A simple model of DMS oxidation was used to estimate the ocean to atmosphere flux rate, and this was found to be within the range of previous estimates, with a mean value of 1011 ng(S)m-2h-1.

Original languageEnglish
Pages (from-to)1895-1906
Number of pages12
JournalAtmospheric Environment
Volume30
Issue number10-11
DOIs
Publication statusPublished - May 1996
Externally publishedYes
EventProceedings of the 1994 Joint 8th CACGP and 2nd IGAC Conference on Global Atmospheric Chemistry - Fuji Yoshida, Jpn
Duration: 5 Sep 19949 Sep 1994

Keywords

  • Aerosol
  • Antarctica
  • Dimethyl sulfide

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